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Zefeng Ren
State-to-State Dynamical Research in the FH2 Reaction System
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2949768State-to-State Dynamical Research in the FH2 Reaction Systemhttps://www.gandhi.com.mx/state-to-state-dynamical-research-in-the-f-h2-reaction-system-9783642397561/phttps://gandhi.vtexassets.com/arquivos/ids/2957700/7e5fef5b-0b28-4b72-aaaa-327963ed2ef3.jpg?v=6383846845032000009621069MXNSpringer Berlin HeidelbergInStock/Ebooks/<p>This thesis addresses two important and also challenging issues in the research of chemical reaction dynamics of FH2 system. One is to probe the reaction resonance and the other is to determine the extent of the breakdown of the Born-Oppenheimer approximation (BOA) experimentally. The author introduces a state-of-the-art crossed molecular beam-scattering apparatus using a hydrogen atom Rydberg "tagging" time-of-flight method, and presents thorough state-to-state experimental studies to address the above issues. The author also describes the observation of the Feshbach resonance in the FH2 reaction, a precise measurement of the differential cross section in the FHD reaction, and validation of a new accurate potential energy surface with spectroscopic accuracy. Moreover, the author determines the reactivity ratio between the ground state F(2P3/2) and the excited state F(2P1/2) in the FD2 reaction, and exploits the breakdown of BOA in the low collision energy.</p>...2885954State-to-State Dynamical Research in the FH2 Reaction System9621069https://www.gandhi.com.mx/state-to-state-dynamical-research-in-the-f-h2-reaction-system-9783642397561/phttps://gandhi.vtexassets.com/arquivos/ids/2957700/7e5fef5b-0b28-4b72-aaaa-327963ed2ef3.jpg?v=638384684503200000InStockMXN99999DIEbook20139783642397561_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9783642397561_<p>This thesis addresses two important and also challenging issues in the research of chemical reaction dynamics of FH2 system. One is to probe the reaction resonance and the other is to determine the extent of the breakdown of the Born-Oppenheimer approximation (BOA) experimentally. The author introduces a state-of-the-art crossed molecular beam-scattering apparatus using a hydrogen atom Rydberg tagging time-of-flight method, and presents thorough state-to-state experimental studies to address the above issues. The author also describes the observation of the Feshbach resonance in the FH2 reaction, a precise measurement of the differential cross section in the FHD reaction, and validation of a new accurate potential energy surface with spectroscopic accuracy. Moreover, the author determines the reactivity ratio between the ground state F(2P3/2) and the excited state F(2P1/2) in the FD2 reaction, and exploits the breakdown of BOA in the low collision energy.</p>(*_*)9783642397561_<p>This thesis addresses two important and also challenging issues in the research of chemical reaction dynamics of FH2 system. One is to probe the reaction resonance and the other is to determine the extent of the breakdown of the Born-Oppenheimer approximation (BOA) experimentally. The author introduces a state-of-the-art crossed molecular beam-scattering apparatus using a hydrogen atom Rydberg "tagging" time-of-flight method, and presents thorough state-to-state experimental studies to address the above issues. The author also describes the observation of the Feshbach resonance in the FH2 reaction, a precise measurement of the differential cross section in the FHD reaction, and validation of a new accurate potential energy surface with spectroscopic accuracy. Moreover, the author determines the reactivity ratio between the ground state F(2P3/2) and the excited state F(2P1/2) in the FD2 reaction, and exploits the breakdown of BOA in the low collision energy.</p>...9783642397561_Springer Berlin Heidelberglibro_electonico_c8d37b3f-e79b-3d47-9594-61ea86f42d97_9783642397561;9783642397561_9783642397561Zefeng RenInglésMéxico2013-11-09T00:00:00+00:00Springer Berlin Heidelberg